Bitla, Yugandhar ; Kaul, S. N. ; Fernandez Barquin, L. ; Gutierrez, J. ; Barandiaran, J. M. ; Pena, A. (2010) Observation of isotropic-dipolar to isotropic-Heisenberg crossover in Co- and Ni-substituted manganites New Journal of Physics, 12 . 093039_1-093039_23. ISSN 1367-2630
|
PDF
- Publisher Version
2MB |
Official URL: http://iopscience.iop.org/1367-2630/12/9/093039
Related URL: http://dx.doi.org/10.1088/1367-2630/12/9/093039
Abstract
High-precision ac susceptibility data have been taken on the La0.7Pb0.3Mn1-y(Co, Ni)yO3 (y=0, 0.1, 0.2 and 0.3) manganite system over a wide range of amplitudes and frequencies of the ac driving field in a temperature range that embraces the critical region near the ferromagnetic (FM)-paramagnetic (PM) phase transition (occurring at the Curie point TC). Elaborate data analysis was performed that (i) enabled the first observation of a crossover from a three-dimensional (3D; d=3) isotropic long-range dipolar asymptotic critical behavior to a d=3 isotropic short-range Heisenberg critical regime as the temperature is raised from TC in the compositions y≠0 (no such crossover is observed in the parent compound, y=0) and (ii) brought out clearly the importance of dipole-dipole interactions between the eg electron spins and/or between eg-t2g electron spins in establishing long-range FM order in the insulating state. The final charge and spin states of Co and Ni ions, substituting for the Mn3+ and/or Mn4+ ions, are arrived at by using a scenario of substitution that is consistent not only with the present results but also with the previously published structural, thermo-gravimetric, bulk magnetization, dc magnetic susceptibility and electrical resistivity data on the same system. The marked similarity seen between the magnetic behavior of the manganite system in question and the quenched random-exchange ferromagnets, within and outside the critical region, suggests that the percolation model forms an adequate description of the FM metal-to-PM insulator transition.
Item Type: | Article |
---|---|
Source: | Copyright of this article belongs to Institute of Physics Publishing. |
ID Code: | 29958 |
Deposited On: | 23 Dec 2010 03:55 |
Last Modified: | 17 May 2016 12:43 |
Repository Staff Only: item control page