Chakraborty, Rayan ; Sim, Kyu Min ; Shrivastava, Megha ; Adarsh, K. V. ; Chung, Dae Sung ; Nag, Angshuman (2019) Colloidal Synthesis, Optical Properties, and Hole Transport Layer Applications of Cu2BaSnS4 (CBTS) Nanocrystals ACS Applied Energy Materials, 2 (5). pp. 3049-3055. ISSN 2574-0962
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Official URL: https://doi.org/10.1021/acsaem.9b00473
Related URL: http://dx.doi.org/10.1021/acsaem.9b00473
Abstract
Cu2BaSnS4 (CBTS) is an emerging earth-abundant and environmentally benign semiconductor. However, there has been no prior report of colloidal CBTS nanocrystals. Here we developed a colloidal synthesis of CBTS nanocrystals by rational design. Photophysical properties of these nanocrystals are elucidated using photoluminescence and ultrafast transient absorption spectroscopy. Finally, thin films of CBTS nanocrystals grown at room temperature are used as the hole transport layer (HTL) in an organic photodiode yielding a high peak specific detectivity (>3.2 × 1012 Jones) with low noise equivalent power (9.20 × 10-14 W Hz0.5). These results suggest that our colloidal CBTS nanocrystals have potential for optoelectronic applications.
| Item Type: | Article |
|---|---|
| Source: | Copyright of this article belongs to American Chemical Society. |
| Keywords: | Metal sulfides; Cu2BaSnS4 nanocrystals; Colloidal semiconductor nanocrystals; Ultrafast carrier dynamics; Hole transport layer; Pphotodiode. |
| ID Code: | 142156 |
| Deposited On: | 11 Jan 2026 05:40 |
| Last Modified: | 11 Jan 2026 05:40 |
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