Paul, Amit K. ; Adhikari, Satrajit ; Mukhopadhyay, Debasis ; Halász, Gabor J. ; Vibók, Ágnes ; Baer, Roi ; Baer, Michael (2009) Photodissociation of H2+ upon exposure to an intense pulsed photonic fock state The Journal of Physical Chemistry A, 113 (26). pp. 7331-7337. ISSN 1089-5639
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Official URL: http://doi.org/10.1021/jp811269g
Related URL: http://dx.doi.org/10.1021/jp811269g
Abstract
Producing and controlling nonclassical light states are now the subject of intense experimental efforts. In this paper we consider the interaction of such a light state with a small molecule. Specifically, we develop the theory and apply it numerically to calculate in detail how a short pulse of nonclassical light, such as the high intensity Fock state, induces photodissociation in H2+. We compare the kinetic energy distributions and photodissociation yields with the analogous results of quasi-classical light, namely a coherent state. We find that Fock-state light decreases the overall probability of dissociation for low vibrational states of H2+ as well as the location of peaks and line shapes in the kinetic energy distribution of the nuclei.
| Item Type: | Article |
|---|---|
| Source: | Copyright of this article belongs to American Chemical Society. |
| ID Code: | 136277 |
| Deposited On: | 20 May 2025 07:09 |
| Last Modified: | 20 May 2025 07:09 |
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