Correlation between structural, transport, and magnetic properties in Sm1−xAxMnO3 (A=Sr,Ca)

Hassen, A. ; Mandal, P. (2007) Correlation between structural, transport, and magnetic properties in Sm1−xAxMnO3 (A=Sr,Ca) Journal of Applied Physics, 101 (11). p. 113917. ISSN 0021-8979

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Official URL: http://doi.org/10.1063/1.2744476

Related URL: http://dx.doi.org/10.1063/1.2744476

Abstract

Transport, magnetic, and structural properties of Sm1−xAxMnO3, where A is Ca and Sr, have been investigated systematically over the range of doping 0≤x≤0.52. For x<0.30, both systems are ferromagnetic (FM) insulator, and the resistivity (ρ) can be described well by polaron hopping model. Above x=0.30, Sr-doped compounds exhibit large negative magnetioresistance (MR) in the FM metallic state and charge/orbital ordering over a narrow doping range around x=0.50. On the other hand, Ca-doped system does not show any insulator to metal transition and MR, possibly due to the smaller average A-site cationic radius ⟨r⟩ than that for Sr-doped one. The magnetic ground state of Ca-doped system changes from FM to canted antiferromagnetic above x=0.30. A strong coupling between transport, magnetic, and structural properties has been established from this study. The results are summarized in (x−T) phase diagrams.

Item Type:Article
Source:Copyright of this article belongs to American Institute of Physics.
ID Code:122860
Deposited On:19 Aug 2021 10:15
Last Modified:19 Aug 2021 10:15

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