Optical nonlinearity in a mode-locking dye: optical limiting and four wave mixing

Kumar, G.Ravindra ; Rajgara, F.A. ; Rangwala, S.A. (1995) Optical nonlinearity in a mode-locking dye: optical limiting and four wave mixing Chemical Physics Letters, 245 (2-3). pp. 287-291. ISSN 0009-2614

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Official URL: http://doi.org/10.1016/0009-2614(95)01007-V

Related URL: http://dx.doi.org/10.1016/0009-2614(95)01007-V

Abstract

We report the optical nonlinearity resonantly induced by picosecond laser excitation in Kodak 9740 mode-locking dye. The observed nonlinearity is due to the participation of high-lying singlet states. The specific processes studied are optical limiting and phase conjugation. We infer that the mechanism underlying the limiting behaviour is due to two-photon absorption, and obtain a value for the two-photon absorption coefficient β. Further, we report the intensity dependence of the phase conjugate signal and obtain the corresponding third-order susceptibility.

Item Type:Article
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ID Code:121127
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