Two-dimensional ferromagnetic ordering in a metal–organic multilayer structure

Abstract

We demonstrate, using spin polarized neutron reflectivity measurements, that one can form a large stack of magnetically decoupled spin-membranes of Gadolinium ions and reduce the effect of the substrate substantially to study short-range Two-dimensional (2D) ferromagnetic ordering. No spontaneous magnetization was observed in these membranes as the magnetic field was applied along an in-plane direction. The results are consistent with theoretical predictions of 2D in-plane spin systems having strong interplay of exchange, magneto-crystalline anisotropy and dipolar interactions. These metal–organic multilayer films will enable us to verify various theoretical predictions regarding spin-fluctuations in 2D systems using conventional magnetic measurements and neutron scattering studies.