The phase of second-harmonic light generated at an interface and its relation to absolute molecular orientation

Kemnitz, K. ; Bhattacharyya, K. ; Hicks, J. M. ; Pinto, G. R. ; Eisenthal, B. ; Heinz, T. F. (1986) The phase of second-harmonic light generated at an interface and its relation to absolute molecular orientation Chemical Physics Letters, 131 (4-5). pp. 285-290. ISSN 0009-2614

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Official URL: http://www.sciencedirect.com/science/article/pii/0...

Related URL: http://dx.doi.org/10.1016/0009-2614(86)87152-4

Abstract

Measurement of the absolute phase of the surface second-harmonic light field with respect to the pump field, i.e. the phase of the surface non-linear susceptibility, is described. From such studies the absolute orientation of surface molecules can be determined. In the present work the liquid/vapor interface of an aqueous phenol solution was investigated.

Item Type:Article
Source:Copyright of this article belongs to Elsevier Science.
ID Code:77192
Deposited On:10 Jan 2012 07:42
Last Modified:10 Jan 2012 07:42

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