Chandrasekhar, S. ; Rambabu, Ch. ; Shyamsunder, T. (2007) Total synthesis of aculeatins A and B via a tethered oxa-Michael approach Tetrahedron Letters, 48 (27). pp. 4683-4685. ISSN 0040-4039
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Official URL: http://www.sciencedirect.com/science/article/pii/S...
Related URL: http://dx.doi.org/10.1016/j.tetlet.2007.05.026
Abstract
A stereocontrolled total synthesis of aculeatins A and B has been achieved in eight steps and in 15% overall yield. The key feature of this synthetic approach is the application of a Marouka allylation and tethered intramolecular oxa-Michael reaction to install the required stereocentres on the tetrahydropyran ring.
| Item Type: | Article |
|---|---|
| Source: | Copyright of this article belongs to Elsevier Science. |
| Keywords: | Aculeatin; Marouka Allylation; Oxa-michael Reaction; Spirocyclic Natural Products |
| ID Code: | 62371 |
| Deposited On: | 22 Sep 2011 03:32 |
| Last Modified: | 22 Sep 2011 03:32 |
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