Transient behaviour of activationless electronic relaxation in solution

Jayannavar, A. M. (1992) Transient behaviour of activationless electronic relaxation in solution Chemical Physics Letters, 199 (1-2). pp. 149-152. ISSN 0009-2614

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Official URL: http://linkinghub.elsevier.com/retrieve/pii/000926...

Related URL: http://dx.doi.org/10.1016/0009-2614(92)80062-G

Abstract

We report a theoretical study of transient behaviour of barrierless electronic reactions in solution. We have generalized the early theory of Oster and Nishijima to the low-friction and small-time domain. An analytical form for the decay of the integrated excited state is derived. We point out the strong friction and temperature dependence of the decay rate in the transient domain.

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