Combined transparency and optical nonlinearity enhancement in flexible covalent multimers by operating through-space interactions between dipolar chromophores

Parthasarathy, Venkatakrishnan ; Pandey, Ravindra ; Terenziani, Francesca ; Das, Puspendu K. ; Blanchard-Desce, Mireille (2014) Combined transparency and optical nonlinearity enhancement in flexible covalent multimers by operating through-space interactions between dipolar chromophores Physical Chemistry Chemical Physics, 16 (19). p. 9096. ISSN 1463-9076

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Official URL: http://doi.org/10.1039/c4cp00715h

Related URL: http://dx.doi.org/10.1039/c4cp00715h

Abstract

Subtle manipulation of mutual repulsion and polarisation effects between polar and polarisable chromophores forced in closed proximity allows achieving major (100%) enhancement of the first hyperpolarisability together with increased transparency, breaking the well-known nonlinearity–transparency trade-off paradigm.

Item Type:Article
Source:Copyright of this article belongs to Royal Society of Chemistry.
ID Code:131588
Deposited On:07 Dec 2022 08:05
Last Modified:07 Dec 2022 08:05

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